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Space view of the decadal variation for typical air pollutants in the Pearl River Delta (PRD) region

Zifeng WANG, Min SHAO, Liangfu CHEN, Minghui TAO, Liuju ZHONG, Duohong CHEN, Meng FAN, Yang WANG, Xinhui WANG

《环境科学与工程前沿(英文)》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0853-y

摘要: Spatial and temporal trends of the typical pollutants in PRD viewed from space. Comparisons of the satellite retrievals with the collocated in situ data are given. Among different MCs, the control measures applied in PRD are the most effective. The unique HCHO trends imply significant contribution from the biogenic origins. The Pearl River Delta (PRD) is one of the most industrialized, urbanized and populated regions in China, and thus has been long suffering from severe air pollutions. Space data provide a unique perspective for investigating the atmospheric environment at a regional scale. By utilizing multiple satellite retrievals from 2005 to 2013, this study presented, for the first time, the spatial patterns and temporal trends of typical air pollutants over PRD and its vicinity. As viewed from space, aerosol optical depth (AOD), NO2 and SO2 all had their higher values at the central part of PRD, and showed clear descending gradients as moving to the outskirt of this region. As to the inter-annual variation, all these pollutants had decreasing trends in PRD during the study period, which generally agreed with the relevant in situ measurements. However, the satellite retrievals differed from ground measurements when addressing NO2 and SO2 in the vicinity of PRD. This work also provides the inter-comparison among PRD and three other metropolitan clusters in China: PRD had relatively high AOD, moderate NO2 and low SO2 levels, and it was the only region achieving the effective reduction of NO2 and SO2 during last decade. Unlike the previous three pollutants, HCHO observed by satellite showed very special patterns: it had a relatively homogeneous spatial distribution over both of PRD and its vicinity, and presented an opposite increasing trend from 2005 to 2010. Moreover, PRD had the highest HCHO level among all the metropolitan clusters, hinting a considerable contribution of biogenic origins of HCHO in PRD.

关键词: The Pearl River Delta (PRD)     Satellite monitoring     Regional air quality     Long-term trend     HCHO    

Photochemical indicators of ozone sensitivity: application in the Pearl River Delta, China

Lyumeng Ye,Xuemei Wang,Shaofeng Fan,Weihua Chen,Ming Chang,Shengzhen Zhou,Zhiyong Wu,Qi Fan

《环境科学与工程前沿(英文)》 2016年 第10卷 第6期 doi: 10.1007/s11783-016-0887-1

摘要: The distribution of NO - and VOC-sensitive regimes in the PRD are identified. The effectiveness of six popular chemical indicators for discriminating O sensitivity regimes is evaluated. Threshold levels for HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO were derived and verified. The indicators H O /HNO and H O /NO performed best and maintained relatively stable threshold levels. Surface O production has a highly nonlinear relationship with its precursors. The spatial and temporal heterogeneity of O -NO -VOC-sensitivity regimes complicates the control- decision making. In this paper, the indicator method was used to establish the relationship between O sensitivity and assessment indicators. Six popular ratios indicating ozone-precursor sensitivity, HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO , and H O /NO , were evaluated based on the distribution of NO - and VOC-sensitive regimes. WRF-Chem was used to study a serious ozone episode in fall over the Pearl River Delta (PRD). It was found that the south-west of the PRD is characterized by a VOC-sensitive regime, while its north-east is NO -sensitive, with a sharp transition area between the two regimes. All indicators produced good representations of the elevated ozone hours in the episode on 6 November 2009, with H O /HNO being the best indicator. The threshold sensitivity levels for HCHO/NO , H O /HNO , O /NO , O /NO , O /HNO , and H O /NO were estimated to be 0.41, 0.55, 10.2, 14.0, 19.1, and 0.38, respectively. Threshold intervals for the indicators H O /HNO , O /NO , O /NO , O /HNO , and H O /NO were able to identify more than 95% of VOC- and NO -sensitive grids. The ozone episode on 16 November 16 2008 was used to independently verify the results, and it was found that only H O /HNO and H O /NO were able to differentiate the ozone sensitivity regime well. Hence, these two ratios are suggested as the most appropriate indicators for identifying fall ozone sensitivity in the PRD. Since the species used for indicators have seasonal variation, the utility of those indicators for other seasons should be investigated in the future work.

关键词: Ozone     Pearl River Delta (PRD)     Sensitivity regime     Photochemical indicator     Threshold levels    

Source attribution for mercury deposition with an updated atmospheric mercury emission inventory in the PearlRiver Delta Region, China

Jiajun Liu, Long Wang, Yun Zhu, Che-Jen Lin, Carey Jang, Shuxiao Wang, Jia Xing, Bin Yu, Hui Xu, Yuzhou Pan

《环境科学与工程前沿(英文)》 2019年 第13卷 第1期 doi: 10.1007/s11783-019-1087-6

摘要:

Estimated anthropogenic Hg emission was 11.9 tons in Pearl River Delta for 2014.

Quantifying contributions of emission sources helps to provide control strategies.

More attentions should be paid to Hg deposition around the large point sources.

Power plant, industrial source and waste incinerator were priorities for control.

A coordinated regional Hg emission control was important for controlling pollution.

关键词: Emission inventory     Mercury deposition     Pearl River Delta (PRD)     Source attribution     Control strategy    

Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

《环境科学与工程前沿(英文)》 2016年 第10卷 第1期   页码 53-62 doi: 10.1007/s11783-014-0728-z

摘要: Understanding the trends in PM levels is essential for formulating clean air plans. This paper analyzes PM data from various published sources for the years 2000 to 2010 in the Pearl River Delta Economic Zone (PRDEZ). The long-term variation in PM mass concentration is analyzed. Results show that PM , organic carbon (OC), elemental carbon (EC), and show a similar trend, increasing before 2005 and then decreasing slightly. The annual average PM concentration ranges from 49.1 μg·m in 2000 to 64.3 μg·m in 2010, with a peak of 84.1 μg·m in 2004. None of these 11 years meets the new National Ambient Air Quality standard (NAAQS) for PM (35 μg·m ). Overall average concentrations of OC, EC, and are 13.0, 6.5, and 11.8 μg·m , respectively. and respectively have concentrations of 1.5 μg·m and 2.9 μg·m in 2000 and 6.4 μg·m and 5.3 μg·m in 2010, with a statistically significant average annual trend of+ 0.2 μg·m ·yr and+ 0.1 μg·m ·yr . In certain geographic regions, OC and EC contribute most of the PM , while in other regions secondary water-soluble ions are more important. In general, OC and are the dominant components of PM , contributing 20.6% and 18.6%, respectively. These results provide, for the first time, a better understanding of the long-term PM characteristics and trends, on a species-by-species basis, in the PRDEZ. The results indicate that PM abatement needs to prioritize secondary species.

关键词: long-term trends     fine particulate matter     chemical components     Pearl River Delta Economic Zone (PRDEZ)    

Characterization of submicron aerosols in the urban outflow of the central Pearl River Delta region of

Zhaoheng GONG, Zijuan LAN, Lian XUE, Liwu ZENG, Lingyan HE, Xiaofeng HUANG

《环境科学与工程前沿(英文)》 2012年 第6卷 第5期   页码 725-733 doi: 10.1007/s11783-012-0441-8

摘要: Submicron aerosol particles (with aerodynamic diameters less than 1 μm, PM ) were sampled and measured in Heshan, an urban outflow site of Guangzhou megacity in Pearl River Delta in South China, using an Aerodyne High-Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS) in November 2010 during 2010 Guangzhou Asian Games. The mean PM mass concentration measured was 47.9±17.0 μg·m during the campaign, with organic aerosol (OA) and sulfate being the two dominant species, accounting for 36.3% and 20.9% of the total mass, respectively, followed by black carbon (17.1%, measured by an aethalometer), nitrate (12.9%), ammonium (9.6%) and chloride (3.1%). The average size distributions of the species (except black carbon) were dominated by an accumulation mode peaking at ~550 nm. Calculations based on high-resolution organic mass spectrum showed that, C, H, O and N on average contributed 58.1%, 7.3%, 30.7%, and 3.9% to the total organic mass, respectively. The average ratio of organic mass over organic carbon mass (OM/OC) was 1.73±0.08. Four components of OA were identified by the Positive Matrix Factorization (PMF) analysis, including a hydrocarbon-like (HOA), a biomass burning (BBOA) and two oxygenated (SV-OOA and LV-OOA) organic aerosol components, which on average accounted for 18.0%, 14.3%, 28.8% and 38.9% of the total organic mass, respectively.

关键词: organic aerosol     high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS)     positive matrix factorization    

珠江三角洲流域环境污染联合防治机制研究

张英民,李开明,刘爱萍

《中国工程科学》 2010年 第12卷 第6期   页码 71-74

摘要:

针对珠江三角洲流域河网众多,城际间联系密切,环境污染呈区域性分布的特征,提出珠江三角洲流域污染联合防治机制。对于流域环境污染防治积极推行环境污染防治联合规划、推进环境污染防治联合整治、强化流域环境污染监督管理的联合执法力度,使珠江三角洲地区的环境污染状况得到有效扼制。

关键词: 珠江三角洲     流域环境污染     联合防治     机制    

珠江三角洲地区生态文明建设提升战略研究

王金南 ,蒋洪强 ,吴文俊 ,刘年磊 ,段扬 ,王明旭

《中国工程科学》 2022年 第24卷 第6期   页码 154-163 doi: 10.15302/J-SSCAE-2022.06.014

摘要:

生态文明建设是国家发展战略,研究经济发达地区生态文明建设的经验模式与提升策略,对发挥带动和示范效应、推 进全国生态文明建设具有重要意义。本文以珠江三角洲(珠三角)地区的生态文明建设为案例,系统梳理了生态空间格局、 生态环境质量、生态文明制度、经济环境协调发展等方面取得的成效,总结提炼了生态文明建设的创新模式;在深入分析区 域生态文明建设面临挑战的基础上,针对性提出了发展目标与发展路径,以期为我国经济发达地区的生态文明建设提供基本 参照。研究建议,提升国土空间保护修复水平,推动珠三角地区率先实现碳排放达峰,以科技创新引领绿色低碳高质量发 展,促进天蓝地绿水清,使环境得到持续改善,营造美丽宜居与生态文明新风尚,以此构建生态文明制度创新高地。

关键词: 生态文明;珠江三角洲;建设模式;生态环境;碳排放达峰;制度创新    

能源革命推动珠江三角洲开放发展研究

呼和涛力,骆志刚,袁汝玲,孙富安,陈勇

《中国工程科学》 2021年 第23卷 第1期   页码 52-59 doi: 10.15302/J-SSCAE-2021.01.009

摘要:

珠江三角洲是我国改革开放的先行地区,在新形势下因地制宜地推进能源革命,对推动珠江三角洲地区的经济、能源与生态环境的协调可持续发展具有重要意义。本文综合分析珠江三角洲地区各类能源供给与消费特点,深入探讨能源革命推动珠江三角洲开放发展所面临的挑战,结合珠江三角洲地区能源转型发展需求,提出了能源革命推动珠江三角洲的开放发展所采取的相关措施及建议。研究得出珠江三角洲需要依托“一带一路”与粤港澳大湾区建设,打造国家油气储备基地和可再生能源基地,实施能源消费总量与强度“双控”,增强能源技术开发与科技创新,以能源革命推动珠江三角洲地区进入绿色低碳高质量发展阶段。

关键词: 能源革命,开放发展,珠江三角洲,粤港澳大湾区    

Energy internet in the Yangtze River Delta: opportunities, challenges, and suggestions

Zheng YAN, Jiayi HU

《能源前沿(英文)》 2018年 第12卷 第4期   页码 484-492 doi: 10.1007/s11708-018-0600-0

摘要:

Energy internet is an Internet of Things (IoT) based network, which combines the multi-energy flows and the information flows. In this review, the opportunities and the challenges posed to developing energy internet in the Yangtze River Delta are analyzed concerning detailed analysis of its advantages in various aspects and problems of its energy systems. Then the framework of energy internet in the Yangtze River Delta is constructed, according to which specific suggestions are also provided. This review is dedicated to helping the policy makers to draw the roadmap of future-oriented energy internet.

关键词: energy internet     opportunities     challenges     suggestions     the Yangtze River Delta    

典型城市群的市域生态文明水平评估研究

杨娇,张林波,罗上华,解钰茜,李芬,

《中国工程科学》 2017年 第19卷 第4期   页码 54-59 doi: 10.15302/J-SSCAE-2017.04.009

摘要:

为评估和反映我国生态文明发展水平,结合联合国2030年可持续发展议程和国家生态文明建设目标,构建了以环境质量改善为核心的生态文明发展指标体系。基于市域评估单元,采用双目标渐进赋分,评估了京津冀、长三角和珠三角三个城市群的生态文明发展水平。结果表明,珠三角城市群生态文明发展水平最高,均值为69.95;其次是长三角城市群,均值为67.61,最后是京津冀城市群,均值为59.04。三个城市群生态文明发展水平的短板都体现在绿色环境领域。城市生态文明发展水平评估,揭示其生态文明建设的短板,为城市提升生态文明发展水平指明了方向。

关键词: 生态文明发展水平     京津冀城市群     长三角城市群     珠三角城市群     双目标渐进法    

Occurrence, removal, and environmental risks of pharmaceuticals in wastewater treatment plants in south China

Huang Huang, Jie Wu, Jian Ye, Tingjin Ye, Jia Deng, Yongmei Liang, Wei Liu

《环境科学与工程前沿(英文)》 2018年 第12卷 第6期 doi: 10.1007/s11783-018-1053-8

摘要:

Five pharmaceuticals were detected in wastewater treatment plants in southern China.

Biological treatment was the most effective process for PhACs removal.

Metoprolol showed negative removal during secondary treatment process.

The pharmaceuticals studied posed a low environmental risk to aquatic ecosystems.

关键词: Pharmaceuticals     Wastewater treatment     Pearl River Delta     Occurrence     Removal     Risk assessment    

Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region

《环境科学与工程前沿(英文)》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1714-0

摘要:

● The emission reduction causes significant change in organic aerosol composition.

关键词: Emission control     Secondary organic aerosol     Atmospheric oxidizing capacity     Holiday effects     COVID-19 lockdown    

PPCPs in a drinking water treatment plant in the Yangtze River Delta of China: Occurrence, removal and

Xinshu Jiang, Yingxi Qu, Liquan Liu, Yuan He, Wenchao Li, Jun Huang, Hongwei Yang, Gang Yu

《环境科学与工程前沿(英文)》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1109-4

摘要:

• 39 PPCPs were investigated at a DWTP using the Yangtze River as its water source.

• Grab and continuous sampling were conducted for the comparison of data consistency.

• Ketoprofen & carbamazepine can be risk management indicators because of the high RQ.

关键词: PPCPs     DWTP     Human health risk assessment    

CONCENTRATIONS AND FLUXES OF DISSOLVED NUTRIENTS IN THE YANGTZE RIVER: LONG-TERM TRENDS AND ECOLOGICAL

《农业科学与工程前沿(英文)》 2021年 第8卷 第4期   页码 559-567 doi: 10.15302/J-FASE -2020344

摘要:

Intensifying human activity in the Yangtze River basin has substantially increased nutrient concentrations in the Yangtze River Estuary, leading to degradation of the coastal environment. Analysis of nutrient determinations published over the past 50 years reveals a gradual decreasing trend in the concentrations and fluxes of dissolved silicate (DSi). However, both dissolved inorganic nitrogen (DIN) and dissolved inorganic phosphate (DIP) concentrations have increased significantly since the 1970s. The frequency of and area covered by red tide outbreaks have increased greatly during this period, mainly due to changes in nutrient supply ratios [i.e., N/P (DIN/DIP), N/Si (DIN/DSi), P/Si (DIP/DSi)]. A strong correlation was found between the riverine DIN fluxes and the estimated DIN inputs from the major N sources, particularly fertilizers and atmospheric deposition. The data provide a comprehensive assessment of nutrients in the Yangtze River basin and their ecological impacts and indicate a potentially significant influence of atmospheric deposition on DIN loadings and fluxes.

 

关键词: atmospheric deposition / ecological impacts / nitrogen sources / nutrients / Yangtze delta    

CONCENTRATIONS AND FLUXES OF DISSOLVED NUTRIENTS IN THE YANGTZE RIVER: LONG-TERM TRENDS AND ECOLOGICAL

Yandan FU, Jiahui KANG, Ziyue LI, Xuejun LIU, Wen XU

《农业科学与工程前沿(英文)》 2021年 第8卷 第4期   页码 559-567 doi: 10.15302/J-FASE-2020344

摘要: Intensifying human activity in the Yangtze River Basin (YRB) has substantially increased nutrient concentrations in the Yangtze River Estuary, leading to degradation of the coastal environment. Analysis of nutrient determinations published over the past 50 years reveals a gradual decreasing trend in the concentrations and fluxes of dissolved silicate (DSi). However, both dissolved inorganic nitrogen (DIN) and dissolved inorganic phosphate (DIP) concentrations have increased significantly since the 1970s. The frequency and area covered by red tide outbreaks have increased greatly during this period, mainly due to changes in nutrient supply ratios [i.e., N/P (DIN/DIP), N/Si (DIN/DSi), P/Si (DIP/DSi)]. A strong correlation was found between the riverine DIN fluxes and the estimated DIN inputs from the major N sources, particularly fertilizers and atmospheric deposition. The data provide a comprehensive assessment of nutrients in the YRB and their ecological impacts and indicate a potentially significant influence of atmospheric deposition on DIN loadings and fluxes.

关键词: atmospheric deposition     ecological impacts     nitrogen sources     nutrients     Yangtze River Delta    

标题 作者 时间 类型 操作

Space view of the decadal variation for typical air pollutants in the Pearl River Delta (PRD) region

Zifeng WANG, Min SHAO, Liangfu CHEN, Minghui TAO, Liuju ZHONG, Duohong CHEN, Meng FAN, Yang WANG, Xinhui WANG

期刊论文

Photochemical indicators of ozone sensitivity: application in the Pearl River Delta, China

Lyumeng Ye,Xuemei Wang,Shaofeng Fan,Weihua Chen,Ming Chang,Shengzhen Zhou,Zhiyong Wu,Qi Fan

期刊论文

Source attribution for mercury deposition with an updated atmospheric mercury emission inventory in the PearlRiver Delta Region, China

Jiajun Liu, Long Wang, Yun Zhu, Che-Jen Lin, Carey Jang, Shuxiao Wang, Jia Xing, Bin Yu, Hui Xu, Yuzhou Pan

期刊论文

Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

期刊论文

Characterization of submicron aerosols in the urban outflow of the central Pearl River Delta region of

Zhaoheng GONG, Zijuan LAN, Lian XUE, Liwu ZENG, Lingyan HE, Xiaofeng HUANG

期刊论文

珠江三角洲流域环境污染联合防治机制研究

张英民,李开明,刘爱萍

期刊论文

珠江三角洲地区生态文明建设提升战略研究

王金南 ,蒋洪强 ,吴文俊 ,刘年磊 ,段扬 ,王明旭

期刊论文

能源革命推动珠江三角洲开放发展研究

呼和涛力,骆志刚,袁汝玲,孙富安,陈勇

期刊论文

Energy internet in the Yangtze River Delta: opportunities, challenges, and suggestions

Zheng YAN, Jiayi HU

期刊论文

典型城市群的市域生态文明水平评估研究

杨娇,张林波,罗上华,解钰茜,李芬,

期刊论文

Occurrence, removal, and environmental risks of pharmaceuticals in wastewater treatment plants in south China

Huang Huang, Jie Wu, Jian Ye, Tingjin Ye, Jia Deng, Yongmei Liang, Wei Liu

期刊论文

Response of organic aerosol characteristics to emission reduction in Yangtze River Delta region

期刊论文

PPCPs in a drinking water treatment plant in the Yangtze River Delta of China: Occurrence, removal and

Xinshu Jiang, Yingxi Qu, Liquan Liu, Yuan He, Wenchao Li, Jun Huang, Hongwei Yang, Gang Yu

期刊论文

CONCENTRATIONS AND FLUXES OF DISSOLVED NUTRIENTS IN THE YANGTZE RIVER: LONG-TERM TRENDS AND ECOLOGICAL

期刊论文

CONCENTRATIONS AND FLUXES OF DISSOLVED NUTRIENTS IN THE YANGTZE RIVER: LONG-TERM TRENDS AND ECOLOGICAL

Yandan FU, Jiahui KANG, Ziyue LI, Xuejun LIU, Wen XU

期刊论文